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      Coherent excitation of a single atom to a Rydberg state

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          Abstract

          We present the coherent excitation of a single Rubidium atom to the Rydberg state (58d3/2) using a two-photon transition. The experimental setup is described in detail, as well as experimental techniques and procedures. The coherence of the excitation is revealed by observing Rabi oscillations between ground and Rydberg states of the atom. We analyze the observed oscillations in detail and compare them to numerical simulations which include imperfections of our experimental system. Strategies for future improvements on the coherent manipulation of a single atom in our settings are given.

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          Fast quantum gates for neutral atoms

          , , (2000)
          We propose several schemes for implementing a fast two-qubit quantum gate for neutral atoms with the gate operation time much faster than the time scales associated with the external motion of the atoms in the trapping potential. In our example, the large interaction energy required to perform fast gate operations is provided by the dipole-dipole interaction of atoms excited to low-lying Rydberg states in constant electric fields. A detailed analysis of imperfections of the gate operation is given.
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            Dipole Blockade and Quantum Information Processing in Mesoscopic Atomic Ensembles

            We describe a technique for manipulating quantum information stored in collective states of mesoscopic ensembles. Quantum processing is accomplished by optical excitation into states with strong dipole-dipole interactions. The resulting ``dipole blockade'' can be used to inhibit transitions into all but singly excited collective states. This can be employed for a controlled generation of collective atomic spin states as well as non-classical photonic states and for scalable quantum logic gates. An example involving a cold Rydberg gas is analyzed.
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              Observation of ultralong-range Rydberg molecules.

              Rydberg atoms have an electron in a state with a very high principal quantum number, and as a result can exhibit unusually long-range interactions. One example is the bonding of two such atoms by multipole forces to form Rydberg-Rydberg molecules with very large internuclear distances. Notably, bonding interactions can also arise from the low-energy scattering of a Rydberg electron with negative scattering length from a ground-state atom. In this case, the scattering-induced attractive interaction binds the ground-state atom to the Rydberg atom at a well-localized position within the Rydberg electron wavefunction and thereby yields giant molecules that can have internuclear separations of several thousand Bohr radii. Here we report the spectroscopic characterization of such exotic molecular states formed by rubidium Rydberg atoms that are in the spherically symmetric s state and have principal quantum numbers, n, between 34 and 40. We find that the spectra of the vibrational ground state and of the first excited state of the Rydberg molecule, the rubidium dimer Rb(5s)-Rb(ns), agree well with simple model predictions. The data allow us to extract the s-wave scattering length for scattering between the Rydberg electron and the ground-state atom, Rb(5s), in the low-energy regime (kinetic energy, <100 meV), and to determine the lifetimes and the polarizabilities of the Rydberg molecules. Given our successful characterization of s-wave bound Rydberg states, we anticipate that p-wave bound states, trimer states and bound states involving a Rydberg electron with large angular momentum-so-called trilobite molecules-will also be realized and directly probed in the near future.
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                Author and article information

                Journal
                12 May 2010
                Article
                10.1103/PhysRevA.82.013405
                1005.2153
                62316525-e1c9-4f91-8c5d-01d3379da8ae

                http://arxiv.org/licenses/nonexclusive-distrib/1.0/

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                Phys. Rev. A 82, 013405 (2010)
                quant-ph

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