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      Upper critical field anisotropy in BaFe2-xCoxAs2 single crystals synthesized without flux

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          Abstract

          The upper critical field was measured upto 12 T for three BaFe2-xCoxAs2 single crystals with estimated Co concentrations of x = 0.082, x = 0.117 and x = 0.143. HC2 versus temperature was measured from temperature dependent resistivity, for various applied magnetic fields, H || ab and H || c. The [dHC2/dT]T=Tc, normalized with the corresponding TC, decreases with increasing Co content, for both directions. The anisotropy {\gamma} defined as HC2 || ab / HC2 || c shows a distinct increase with Co content, and its temperature dependence shows a peak close to the TC. Magneto transport measurements, in the spin density wave regions, showed significant negative MR for H || ab and positive MR of H || c in the x = 0.082 sample. The implications of these results are discussed.

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          Effects of Co substitution on thermodynamic and transport properties and anisotropic \(H_{c2}\) in Ba(Fe\(_{1-x}\)Co\(_x\))\(_2\)As\(_2\) single crystals

          Single crystalline samples of Ba(Fe\(_{1-x}\)Co\(_x\))\(_2\)As\(_2\) with \(x < 0.12\) have been grown and characterized via microscopic, thermodynamic and transport measurements. With increasing Co substitution, the thermodynamic and transport signatures of the structural (high temperature tetragonal to low temperature orthorhombic) and magnetic (high temperature non magnetic to low temperature antiferromagnetic) transitions are suppressed at a rate of roughly 15 K per percent Co. In addition, for \(x \ge 0.038\) superconductivity is stabilized, rising to a maximum \(T_c\) of approximately 23 K for \(x \approx 0.07\) and decreasing for higher \(x\) values. The \(T - x\) phase diagram for Ba(Fe\(_{1-x}\)Co\(_x\))\(_2\)As\(_2\) indicates that either superconductivity can exist in both low temperature crystallographic phases or that there is a structural phase separation. Anisotropic, superconducting, upper critical field data (\(H_{c2}(T)\)) show a significant and clear change in anisotropy between samples that have higher temperature structural phase transitions and those that do not. These data show that the superconductivity is sensitive to the suppression of the higher temperature phase transition.
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            Nearly Isotropic superconductivity in (Ba,K)Fe2As2

            Superconductivity was recently observed in the iron-arsenic-based compounds with a superconducting transition temperature (Tc) as high as 56K [1-7], naturally raising comparisons with the high Tc copper oxides. The copper oxides have layered crystal structures with quasi-two-dimensional electronic properties, which led to speculations that reduced dimensionality (that is, extreme anisotropy) is a necessary prerequisite for superconductivity at temperatures above 40 K [8,9]. Early work on the iron-arsenic compounds seemed to support this view [7,10]. Here we report measurements of the electrical resistivity in single crystals of (Ba,K)Fe2As2 in a magnetic field up to 60 T. We find that the superconducting properties are in fact quite isotropic, being rather independent of the direction of the applied magnetic fields at low temperature. Such behaviour is strikingly different from all previously-known layered superconductors [9,11], and indicates that reduced dimensionality in these compounds is not a prerequisite for high-temperature superconductivity. We suggest that this situation arises because of the underlying electronic structure of the iron-arsenide compounds, which appears to be much more three dimensional than that of the copper oxides. Extrapolations of low-field single-crystal data incorrectly suggest a high anisotropy and a greatly exaggerated zero-temperature upper critical field.
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              Author and article information

              Journal
              08 March 2011
              Article
              10.1103/PhysRevB.84.012502
              1103.1476
              fe09806b-ddc5-43cf-99b5-2d30f3cd57dc

              http://arxiv.org/licenses/nonexclusive-distrib/1.0/

              History
              Custom metadata
              Phys. Rev B vol(84) 012502 (2011)
              12 pages 7 figures
              cond-mat.supr-con

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