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      Single-Electron Transfer Living Radical Polymerization Platform to Practice, Develop, and Invent.

      1 , 2 , 1 , 1
      Biomacromolecules
      American Chemical Society (ACS)

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          Abstract

          The most fundamental aspects of single-electron transfer (SET) principles are presented. They are discussed according to different definitions used by expert practitioners and are applied to SET living radical polymerization (SET-LRP) according to the definition of the division of organic chemistry of IUPAC that relies on principles elaborated by Taube, Eberson, Chanon, and Kochi. Additional definitions are also discussed to help clarify for the nonexpert contradictory literature reports. Subsequently, the principles and evolution of SET-LRP together with the methodologies currently available to practice it are discussed. It is expected that this Perspective will be able to help experts and nonexperts practice, develop, and invent new concepts and methodologies for SET-LRP to advance its status and the status of other living radical polymerization methods to the level of the most precise living polymerization methods.

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          Author and article information

          Journal
          Biomacromolecules
          Biomacromolecules
          American Chemical Society (ACS)
          1526-4602
          1525-7797
          Oct 09 2017
          : 18
          : 10
          Affiliations
          [1 ] Roy & Diana Vagelos Laboratories, Department of Chemistry, University of Pennsylvania , Philadelphia, Pennsylvania 19104-6323, United States.
          [2 ] Laboratory of Sustainable Polymers, Department of Analytical Chemistry and Organic Chemistry, Universitat Rovira i Virgili , Tarragona 43007, Spain.
          Article
          10.1021/acs.biomac.7b01131
          28849905
          8eaf1561-8373-4e72-b5ef-b65083261694
          History

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