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      Broadband sensory networks with locally stored responsivities for neuromorphic machine vision

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          Abstract

          As the most promising candidates for the implementation of in-sensor computing, retinomorphic vision sensors can constitute built-in neural networks and directly implement multiply-and-accumulation operations using responsivities as the weights. However, existing retinomorphic vision sensors mainly use a sustained gate bias to maintain the responsivity due to its volatile nature. Here, we propose an ion-induced localized-field strategy to develop retinomorphic vision sensors with nonvolatile tunable responsivity in both positive and negative regimes and construct a broadband and reconfigurable sensory network with locally stored weights to implement in-sensor convolutional processing in spectral range of 400 to 1800 nanometers. In addition to in-sensor computing, this retinomorphic device can implement in-memory computing benefiting from the nonvolatile tunable conductance, and a complete neuromorphic visual system involving front-end in-sensor computing and back-end in-memory computing architectures has been constructed, executing supervised and unsupervised learning tasks as demonstrations. This work paves the way for the development of high-speed and low-power neuromorphic machine vision for time-critical and data-intensive applications.

          Abstract

          Non-volatile modulation of responsivity in positive and negative regimes is realized by ion-induced electrostatic field.

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          Architecture of graphdiyne nanoscale films

          We have demonstrated a methodology to generate large area graphdiyne films with 3.61 cm(2) on the surface of copper via a cross-coupling reaction using hexaethynylbenzene. The device based on graphdiyne films for measurement of electrical property is fabricated and shows conductivity of 2.516 x 10(-4) S m(-1) indicating a semiconductor property.
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            A non-volatile organic electrochemical device as a low-voltage artificial synapse for neuromorphic computing

            A neuromorphic device based on the stable electrochemical fine-tuning of the conductivity of an organic ionic/electronic conductor is realized. These devices show high linearity, low noise and extremely low switching voltage.
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              In-memory computing with resistive switching devices

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                Author and article information

                Contributors
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: Funding acquisitionRole: ResourcesRole: SoftwareRole: SupervisionRole: ValidationRole: VisualizationRole: Writing - original draftRole: Writing - review & editing
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: Funding acquisitionRole: ResourcesRole: SoftwareRole: ValidationRole: VisualizationRole: Writing - original draftRole: Writing - review & editing
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: Funding acquisitionRole: Project administrationRole: SoftwareRole: SupervisionRole: ValidationRole: VisualizationRole: Writing - original draftRole: Writing - review & editing
                Role: InvestigationRole: Resources
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: Funding acquisitionRole: ResourcesRole: SoftwareRole: ValidationRole: VisualizationRole: Writing - original draftRole: Writing - review & editing
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: Funding acquisitionRole: SoftwareRole: ValidationRole: VisualizationRole: Writing - review & editing
                Role: ConceptualizationRole: InvestigationRole: MethodologyRole: ResourcesRole: Writing - review & editing
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: InvestigationRole: Project administrationRole: ResourcesRole: SoftwareRole: SupervisionRole: ValidationRole: Writing - original draftRole: Writing - review & editing
                Role: ConceptualizationRole: Formal analysisRole: Writing - original draft
                Role: Writing - review & editing
                Role: ConceptualizationRole: Formal analysisRole: Funding acquisitionRole: InvestigationRole: Project administrationRole: SoftwareRole: SupervisionRole: Validation
                Role: ConceptualizationRole: Formal analysisRole: Funding acquisitionRole: MethodologyRole: Project administrationRole: ResourcesRole: SupervisionRole: ValidationRole: VisualizationRole: Writing - original draft
                Journal
                Sci Adv
                Sci Adv
                sciadv
                advances
                Science Advances
                American Association for the Advancement of Science
                2375-2548
                September 2023
                15 September 2023
                : 9
                : 37
                : eadi5104
                Affiliations
                [ 1 ]MOE International Joint Laboratory of Materials Microstructure, Institute for New Energy Materials and Low Carbon Technologies, School of Material Science and Engineering, Tianjin University of Technology, Tianjin 300384, China.
                [ 2 ]The Key Laboratory of Weak Light Nonlinear Photonics, Ministry of Education, School of Physics, Nankai University, Tianjin 300071, China.
                [ 3 ]Key Laboratory of Multifunctional Nanomaterials and Smart Systems Division of Advanced Material, Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences, Suzhou 215123, China.
                [ 4 ]Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China.
                Author notes
                [* ]Corresponding author. Email: chenxd@ 123456nankai.edu.cn (X.-D.C.); lutongbu@ 123456tjut.edu.cn (T.-B.L.); jinzhang@ 123456pku.edu.cn (J.Z.)
                [†]

                These authors contributed equally to this work.

                Author information
                https://orcid.org/0009-0008-8274-3276
                https://orcid.org/0009-0007-4618-5441
                https://orcid.org/0000-0002-0184-3953
                https://orcid.org/0000-0003-3837-7711
                https://orcid.org/0000-0001-9210-156X
                https://orcid.org/0000-0002-6087-4880
                https://orcid.org/0000-0003-3731-8859
                Article
                adi5104
                10.1126/sciadv.adi5104
                10881039
                37713483
                5bce76f9-499b-4863-9ba0-791763b9daba
                Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).

                This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license, which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.

                History
                : 30 April 2023
                : 14 August 2023
                Funding
                Funded by: FundRef http://dx.doi.org/10.13039/501100001809, National Natural Science Foundation of China;
                Award ID: 62274119
                Funded by: FundRef http://dx.doi.org/10.13039/501100001809, National Natural Science Foundation of China;
                Award ID: 51802220
                Funded by: FundRef http://dx.doi.org/10.13039/501100001809, National Natural Science Foundation of China;
                Award ID: 12174207
                Funded by: FundRef http://dx.doi.org/10.13039/501100001809, National Natural Science Foundation of China;
                Award ID: 11974190
                Funded by: the Fundamental Research Funds for the Central Universities;
                Award ID: 010-63233006
                Funded by: the Fundamental Research Funds for the Central Universities;
                Award ID: 010-DK2300010203
                Categories
                Research Article
                Physical and Materials Sciences
                SciAdv r-articles
                Materials Science
                Applied Sciences and Engineering
                Applied Sciences and Engineering
                Custom metadata
                Vivian Hernandez

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