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      Characterization of key aroma compounds and relationship between aroma compounds and sensory attributes in different aroma types of Fu brick tea

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          Highlights

          • Aroma characteristics of Fu brick tea were classified into three types.

          • Key aroma compounds in three aroma types of Fu brick tea were identified.

          • Relationship between aroma compounds and aroma attributes was illuminated.

          Abstract

          Aroma is one of the most important sensory properties of tea. Floral-fungal aroma type, ripe-fungal aroma type and fresh-fungal aroma type were the main aroma types of Fu brick tea by QDA. A total of 112 volatile compounds were identified and quantified in tea samples by HS-SPME/GC–MS analysis. Ten voaltiles in floral-fungal aroma type, eleven voaltiles in ripe-fungal aroma type, and eighteen voaltiles in fresh-fungal aroma type were identified as key aroma compounds for the aroma characteristics formation in three aroma types of Fu brick tea. In addition, PLS analysis revealed that 3,4-dehydro- β-ionone, dihydro- β-ionone, (+)-carotol and linalool oxide were the key contributors to the ‘floral and fruity’ attribute, α-terpineol contributed to ‘woody’ and ‘stale’ attributes, and thirteen aroma compounds related to ‘green’ attribute. Taken together, these findings will provide new insights into the formation mechanism of different aroma characteristics in Fu brick tea.

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          Most cited references40

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          Identification of key odorants responsible for chestnut-like aroma quality of green teas

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            Comparison of Aroma-Active Volatiles in Oolong Tea Infusions Using GC–Olfactometry, GC–FPD, and GC–MS

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              Characterization of the key aroma compounds in Longjing tea using stir bar sorptive extraction (SBSE) combined with gas chromatography-mass spectrometry (GC-MS), gas chromatography-olfactometry (GC-O), odor activity value (OAV), and aroma recombination.

              Longjing tea is the most famous premium green tea, and is regarded as the national tea in China, with its attractive aroma contributing as a prime factor for its general acceptability; however, its key aroma compounds are essentially unknown. In the present study, volatile compounds from Longjing tea were extracted and examined using stir bar sorptive extraction (SBSE) combined with gas chromatography-mass spectrometry (GC-MS). Data obtained from the present study revealed that 151 volatile compounds from 16 different chemical classes were identified by GC-MS analysis. Enols (8096 µg/kg), alkanes (6744 µg/kg), aldehydes (6442 µg/kg), and esters (6161 µg/kg) were the four major chemical classes and accounted for 54% of the total content of volatile compounds. Geraniol (6736 µg/kg) was the most abundant volatile compound in Longjing tea, followed by hexanal (1876 µg/kg) and β-ionone (1837 µg/kg). Moreover, 14 volatile compounds were distinguished as the key aroma compounds of Longjing tea based on gas chromatography-olfactometry (GC-O) analysis, odor activity value (OAV) calculations, and a preliminary aroma recombination experiment, including 2-methyl butyraldehyde, dimethyl sulfoxide, heptanal, benzaldehyde, 1-octen-3-ol, (E, E)-2,4-heptadienal, benzeneacetaldehyde, linalool oxide I, (E, E)-3,5-octadien-2-one, linalool, nonanal, methyl salicylate, geraniol, and β-ionone. This is the first comprehensive report describing the aroma characterizations and the key aroma compounds in Longjing tea using SBSE/GC-MS. The findings from this study contribute to the scientific elucidation of the chemical basis for the aromatic qualities of Longjing tea.
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                Author and article information

                Contributors
                Journal
                Food Chem X
                Food Chem X
                Food Chemistry: X
                Elsevier
                2590-1575
                07 February 2022
                30 March 2022
                07 February 2022
                : 13
                : 100248
                Affiliations
                [a ]Key Laboratory of Tea Science of Ministry of Education, Hunan Agricultural University, Changsha, Hunan 410128, PR China
                [b ]Collaborative Innovation Centre of Utilization of Functional Ingredients from Botanicals, Hunan Agricultural University, Changsha, Hunan 410128, PR China
                [c ]National Research Center of Engineering Technology for Utilization of Functional Ingredients from Botanicals, Hunan Agricultural University, Changsha, Hunan 410128, PR China
                Author notes
                [* ]Corresponding authors at: Key Laboratory of Tea Science of Ministry of Education, Hunan Agricultural University, Changsha, Hunan 410128, PR China. jianan-huang@ 123456hotmail.com liqinvip@ 123456hotmail.com
                Article
                S2590-1575(22)00046-3 100248
                10.1016/j.fochx.2022.100248
                9040021
                35499020
                2a294332-6b5c-4c83-a859-31601eb7d8e7
                © 2022 The Author(s)

                This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).

                History
                : 4 December 2021
                : 25 January 2022
                : 4 February 2022
                Categories
                Article(s) from the Special Issue on Advances in Tea Chemistry, Flavor, Safety and Health by Dr. Xu and Dr. Yin

                benzyl alcohol (pubchem cid: 244),linalool (pubchem cid: 6549),nerolidol (pubchem cid: 5284507),β-ionone (pubchem cid: 5352481),α-terpineol (pubchem cid: 17100),acetophenone (pubchem cid: 7410),(e,z)-2,6-nonadienal (pubchem cid: 643731),hexanal (pubchem cid: 6184),dihydro-β-ionone (pubchem cid: 519382),(e,e)-2,4-nonadienal (pubchem cid: 5283339).,fu brick tea,different aroma types,key aroma compounds,sensory attributes,multivariate statistical analysis

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