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      A flexible ultrasensitive optoelectronic sensor array for neuromorphic vision systems

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          Abstract

          The challenges of developing neuromorphic vision systems inspired by the human eye come not only from how to recreate the flexibility, sophistication, and adaptability of animal systems, but also how to do so with computational efficiency and elegance. Similar to biological systems, these neuromorphic circuits integrate functions of image sensing, memory and processing into the device, and process continuous analog brightness signal in real-time. High-integration, flexibility and ultra-sensitivity are essential for practical artificial vision systems that attempt to emulate biological processing. Here, we present a flexible optoelectronic sensor array of 1024 pixels using a combination of carbon nanotubes and perovskite quantum dots as active materials for an efficient neuromorphic vision system. The device has an extraordinary sensitivity to light with a responsivity of 5.1 × 10 7 A/W and a specific detectivity of 2 × 10 16 Jones, and demonstrates neuromorphic reinforcement learning by training the sensor array with a weak light pulse of 1 μW/cm 2.

          Abstract

          To emulate nature biological processing, highly-integrated ultra-sensitive artificial neuromorphic system is highly desirable. Here, the authors report flexible sensor array of 1024 pixels using combination of carbon nanotubes and perovskite QDs as active matetials, achieving highly responsive device for reinforcement learning.

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          Most cited references52

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          Deep learning.

          Deep learning allows computational models that are composed of multiple processing layers to learn representations of data with multiple levels of abstraction. These methods have dramatically improved the state-of-the-art in speech recognition, visual object recognition, object detection and many other domains such as drug discovery and genomics. Deep learning discovers intricate structure in large data sets by using the backpropagation algorithm to indicate how a machine should change its internal parameters that are used to compute the representation in each layer from the representation in the previous layer. Deep convolutional nets have brought about breakthroughs in processing images, video, speech and audio, whereas recurrent nets have shone light on sequential data such as text and speech.
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            Ultrasensitive photodetectors based on monolayer MoS2.

            Two-dimensional materials are an emerging class of new materials with a wide range of electrical properties and potential practical applications. Although graphene is the most well-studied two-dimensional material, single layers of other materials, such as insulating BN (ref. 2) and semiconducting MoS2 (refs 3, 4) or WSe2 (refs 5, 6), are gaining increasing attention as promising gate insulators and channel materials for field-effect transistors. Because monolayer MoS2 is a direct-bandgap semiconductor due to quantum-mechanical confinement, it could be suitable for applications in optoelectronic devices where the direct bandgap would allow a high absorption coefficient and efficient electron-hole pair generation under photoexcitation. Here, we demonstrate ultrasensitive monolayer MoS2 phototransistors with improved device mobility and ON current. Our devices show a maximum external photoresponsivity of 880 A W(-1) at a wavelength of 561 nm and a photoresponse in the 400-680 nm range. With recent developments in large-scale production techniques such as liquid-scale exfoliation and chemical vapour deposition-like growth, MoS2 shows important potential for applications in MoS2-based integrated optoelectronic circuits, light sensing, biomedical imaging, video recording and spectroscopy.
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              Quantum Dot Light-Emitting Diodes Based on Inorganic Perovskite Cesium Lead Halides (CsPbX3 ).

              Novel quantum-dot light-emitting diodes based on all-inorganic perovskite CsPbX3 (X = Cl, Br, I) nanocrystals are reported. The well-dispersed, single-crystal quantum dots (QDs) exhibit high quantum yields, and tunable light emission wavelength. The demonstration of these novel perovskite QDs opens a new avenue toward designing optoelectronic devices, such as displays, photodetectors, solar cells, and lasers.
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                Author and article information

                Contributors
                sqiu2010@sinano.ac.cn
                lixiaoming@njust.edu.cn
                cheng@imr.ac.cn
                dmsun@imr.ac.cn
                Journal
                Nat Commun
                Nat Commun
                Nature Communications
                Nature Publishing Group UK (London )
                2041-1723
                19 March 2021
                19 March 2021
                2021
                : 12
                : 1798
                Affiliations
                [1 ]GRID grid.9227.e, ISNI 0000000119573309, Shenyang National Laboratory for Materials Science, Institute of Metal Research, , Chinese Academy of Sciences, ; Shenyang, China
                [2 ]GRID grid.59053.3a, ISNI 0000000121679639, School of Material Science and Engineering, , University of Science and Technology of China, ; Hefei, China
                [3 ]GRID grid.410579.e, ISNI 0000 0000 9116 9901, College of Materials Science and Engineering, , Nanjing University of Science and Technology, ; Nanjing, China
                [4 ]GRID grid.440637.2, ISNI 0000 0004 4657 8879, School of Physical Science and Technology, , ShanghaiTech University, ; Shanghai, China
                [5 ]GRID grid.412252.2, ISNI 0000 0004 0368 6968, College of Information Science and Engineering, , Northeastern University, ; Shenyang, China
                [6 ]GRID grid.41156.37, ISNI 0000 0001 2314 964X, School of Electronic Science and Engineering, , Nanjing University, ; Nanjing, China
                [7 ]GRID grid.9227.e, ISNI 0000000119573309, Suzhou Institute of Nano-Tech and Nano-Bionics, , Chinese Academy of Sciences, ; Suzhou, China
                [8 ]GRID grid.12527.33, ISNI 0000 0001 0662 3178, Tsinghua-Berkeley Shenzhen Institute, , Tsinghua University, ; Shenzhen, China
                Author information
                http://orcid.org/0000-0002-8778-3831
                http://orcid.org/0000-0001-7126-9224
                http://orcid.org/0000-0001-8975-5626
                http://orcid.org/0000-0001-6965-4940
                http://orcid.org/0000-0002-0260-1059
                http://orcid.org/0000-0002-5387-4241
                http://orcid.org/0000-0003-1552-7940
                Article
                22047
                10.1038/s41467-021-22047-w
                7979753
                33741964
                24236970-afb5-4894-bdab-e7d34593f199
                © The Author(s) 2021

                Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

                History
                : 30 October 2020
                : 25 February 2021
                Funding
                Funded by: FundRef https://doi.org/10.13039/501100001809, National Natural Science Foundation of China (National Science Foundation of China);
                Award ID: 61574143, 51532008, 61704175, 51502304, 22075312, 21773292 and 61874054
                Award Recipient :
                Categories
                Article
                Custom metadata
                © The Author(s) 2021

                Uncategorized
                electronic devices,carbon nanotubes and fullerenes,quantum dots
                Uncategorized
                electronic devices, carbon nanotubes and fullerenes, quantum dots

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