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      Review and Prospect of Single-Shot Ultrafast Optical Imaging by Active Detection

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          Abstract

          In the recent decade, single-shot ultrafast optical imaging by active detection, called single-shot active ultrafast optical imaging (SS-AUOI) here, has made great progress, e.g., with a temporal resolution of 50 fs and a frame rate beyond 10 trillion frames per second. Now, it has become indispensable for charactering the nonrepeatable and difficult-to-reproduce events and revealing the underlying physical, chemical, and biological mechanisms. On the basis of this delightful status, we would like to make a review of SS-AUOI. On the basis of a brief introduction of SS-AUOI, our review starts with discussing its characteristics and then focuses on the survey and prospect of SS-AUOI technology.

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          Compressed sensing

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            Femtochemistry:  Atomic-Scale Dynamics of the Chemical Bond†

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              Isolated single-cycle attosecond pulses.

              We generated single-cycle isolated attosecond pulses around approximately 36 electron volts using phase-stabilized 5-femtosecond driving pulses with a modulated polarization state. Using a complete temporal characterization technique, we demonstrated the compression of the generated pulses for as low as 130 attoseconds, corresponding to less than 1.2 optical cycles. Numerical simulations of the generation process show that the carrier-envelope phase of the attosecond pulses is stable. The availability of single-cycle isolated attosecond pulses opens the way to a new regime in ultrafast physics, in which the strong-field electron dynamics in atoms and molecules is driven by the electric field of the attosecond pulses rather than by their intensity profile.
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                Author and article information

                Journal
                Ultrafast Science
                Ultrafast Sci
                American Association for the Advancement of Science (AAAS)
                2765-8791
                January 2023
                January 2023
                : 3
                Affiliations
                [1 ]Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, Shenzhen Key Lab of Micro-Nano Photonic Information Technology, College of Physics and Optoelectronic Engineering, Shenzhen University, Guangdong 518060, China.
                Article
                10.34133/ultrafastscience.0020
                19308f63-b999-44c1-a08a-3464e72420b9
                © 2023
                History

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