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      Solution‐Processed Perovskite Quantum Dot Quasi‐BIC Laser from Miniaturized Low‐Lateral‐Loss Cavity

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          Abstract

          Laser devices produced via solution‐processed perovskite quantum dots (QDs) offer broad spectral tunability as well as ease of fabrication. Utilizing quasi‐bound states in the continuum (quasi‐BIC) modes, solution‐processed QD laser devices have been demonstrated with a nanostructure coated in a thin‐film gain media configuration. However, light leakage through thin‐film guiding from the cavity side edges becomes more pronounced when shrinking the cavity size, posing challenges for the miniaturization of quasi‐BIC‐based lasers. Here, the fabrication of well‐defined patterns of QDs via a solution process allows them to take advantage of the pattern edges to reduce losses through the cavity edges. A single‐mode BIC laser is reported by using CsPbBr 3 QDs with a narrow linewidth of ≈0.1 nm. Importantly, a miniaturized quasi‐BIC laser is realized with a device size as small as 10 × 10 µm 2, making it the smallest among existing solution‐processed BIC lasers. This work provides a strategy for developing ultra‐compact BIC lasers via solution‐processed gain media.

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          Bound states in the continuum

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            Genesis, challenges and opportunities for colloidal lead halide perovskite nanocrystals

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              Observation of trapped light within the radiation continuum.

              The ability to confine light is important both scientifically and technologically. Many light confinement methods exist, but they all achieve confinement with materials or systems that forbid outgoing waves. These systems can be implemented by metallic mirrors, by photonic band-gap materials, by highly disordered media (Anderson localization) and, for a subset of outgoing waves, by translational symmetry (total internal reflection) or by rotational or reflection symmetry. Exceptions to these examples exist only in theoretical proposals. Here we predict and show experimentally that light can be perfectly confined in a patterned dielectric slab, even though outgoing waves are allowed in the surrounding medium. Technically, this is an observation of an 'embedded eigenvalue'--namely, a bound state in a continuum of radiation modes--that is not due to symmetry incompatibility. Such a bound state can exist stably in a general class of geometries in which all of its radiation amplitudes vanish simultaneously as a result of destructive interference. This method to trap electromagnetic waves is also applicable to electronic and mechanical waves.
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                Author and article information

                Contributors
                (View ORCID Profile)
                Journal
                Advanced Functional Materials
                Adv Funct Materials
                Wiley
                1616-301X
                1616-3028
                June 2024
                February 22 2024
                June 2024
                : 34
                : 26
                Affiliations
                [1 ] School of Engineering The University of Tokyo 7‐3‐1 Hongo Bunkyo‐ku Tokyo 113–8656 Japan
                [2 ] Advanced Research Laboratory, Technology Infrastructure Center, Technology Platform Sony Group Corporation 4‐14‐1 Asahi‐cho Atsugi‐shi 243‐0014 Japan
                [3 ] Research Center for Electronic and Optical Materials National Institute for Materials Science (NIMS) 1‐1 Namiki Tsukuba Ibaraki 305‐0044 Japan
                [4 ] Department of Materials Science and Engineering National Taiwan University No. 1, Sec. 4, Roosevelt Rd. Taipei 10617 Taiwan
                Article
                10.1002/adfm.202314953
                0f651ec8-8f3e-4294-82f8-a0602a33febd
                © 2024

                http://creativecommons.org/licenses/by-nc-nd/4.0/

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