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      Spatiotemporal distribution of ground-level ozone in China at a city level

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      Scientific Reports
      Nature Publishing Group UK
      Environmental impact, Sustainability

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          Abstract

          In recent years, ozone (O 3) pollution in China has shown a worsening trend. Due to the vast territory of China, O 3 pollution is a widespread and complex problem. It is vital to understand the current spatiotemporal distribution of O 3 pollution in China. In this study, we collected hourly data on O 3 concentrations in 338 cities from January 1, 2016, to February 28, 2019, to analyze O 3 pollution in China from a spatiotemporal perspective. The spatial analysis showed that the O 3 concentrations exceeded the limit in seven geographical regions of China to some extent, with more serious pollution in North, East, and Central China. The O 3 concentrations in the eastern areas were usually higher than those in the western areas. The temporal analysis showed seasonal variations in O 3 concentration, with the highest O 3 concentration in the summer and the lowest in the winter. The weekend effect, which occurs in other countries (such as the USA), was found only in some cities in China. We also found that the highest O 3 concentration usually occurred in the afternoon and the lowest was in the early morning. The comprehensive analysis in this paper could improve our understanding of the severity of O 3 pollution in China.

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          Ozone pollution in China: A review of concentrations, meteorological influences, chemical precursors, and effects.

          High concentrations of ozone in urban and industrial regions worldwide have long been a major air quality issue. With the rapid increase in fossil fuel consumption in China over the past three decades, the emission of chemical precursors to ozone-nitrogen oxides and volatile organic compounds-has increased sharply, surpassing that of North America and Europe and raising concerns about worsening ozone pollution in China. Historically, research and control have prioritized acid rain, particulate matter, and more recently fine particulate matter (PM2.5). In contrast, less is known about ozone pollution, partly due to a lack of monitoring of atmospheric ozone and its precursors until recently. This review summarizes the main findings from published papers on the characteristics and sources and processes of ozone and ozone precursors in the boundary layer of urban and rural areas of China, including concentration levels, seasonal variation, meteorology conducive to photochemistry and pollution transport, key production and loss processes, ozone dependence on nitrogen oxides and volatile organic compounds, and the effects of ozone on crops and human health. Ozone concentrations exceeding the ambient air quality standard by 100-200% have been observed in China's major urban centers such as Jing-Jin-Ji, the Yangtze River delta, and the Pearl River delta, and limited studies suggest harmful effect of ozone on human health and agricultural corps; key chemical precursors and meteorological conditions conductive to ozone pollution have been investigated, and inter-city/region transport of ozone is significant. Several recommendations are given for future research and policy development on ground-level ozone.
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            Fine particulate matter (PM2.5) in China at a city level

            This study presents one of the first long term datasets including a statistical summary of PM2.5 concentrations obtained from one-year monitoring in 190 cities in China. We found only 25 out of 190 cities could meet the National Ambient Air Quality Standards of China, and the population-weighted mean of PM2.5 in Chinese cities are 61 μg/m3, ~3 times as high as global population-weighted mean, highlighting a high health risk. PM2.5 concentrations are generally higher in north than in south regions due to relative large PM emissions and unfavorable meteorological conditions for pollution dispersion. A remarkable seasonal variability of PM2.5 is observed with the highest during the winter and the lowest during the summer. Due to the enhanced contributions from dust particles and open biomass burning, high PM2.5 abundances are also found in the spring (in Northwest and West Central China) and autumn (in East China), respectively. In addition, we found the lowest and highest PM2.5 often occurs in the afternoon and evening hours, respectively, associated with daily variation of the boundary layer depth and anthropogenic emissions. The diurnal distribution of the PM2.5-to-CO ratio consistently displays a pronounced peak during the afternoon periods, reflecting a significant contribution of secondary PM formation.
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              Threat to future global food security from climate change and ozone air pollution

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                Author and article information

                Contributors
                gfyang@dlut.edu.cn
                Journal
                Sci Rep
                Sci Rep
                Scientific Reports
                Nature Publishing Group UK (London )
                2045-2322
                29 April 2020
                29 April 2020
                2020
                : 10
                : 7229
                Affiliations
                ISNI 0000 0000 9247 7930, GRID grid.30055.33, Institute of Systems Engineering, , Dalian University of Technology, ; Dalian, China
                Article
                64111
                10.1038/s41598-020-64111-3
                7190652
                32350319
                fd89205d-e687-4c18-8a4b-d121157a26ad
                © The Author(s) 2020

                Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

                History
                : 29 October 2019
                : 20 March 2020
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                © The Author(s) 2020

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                environmental impact,sustainability
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                environmental impact, sustainability

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