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      A general method to synthesize and sinter bulk ceramics in seconds

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          Abstract

          Ceramics are an important class of materials with widespread applications because of their high thermal, mechanical, and chemical stability. Computational predictions based on first principles methods can be a valuable tool in accelerating materials discovery to develop improved ceramics. It is essential to experimentally confirm the material properties of such predictions. However, materials screening rates are limited by the long processing times and the poor compositional control from volatile element loss in conventional ceramic sintering techniques. To overcome these limitations, we developed an ultrafast high-temperature sintering (UHS) process for the fabrication of ceramic materials by radiative heating under an inert atmosphere. We provide several examples of the UHS process to demonstrate its potential utility and applications, including advancements in solid-state electrolytes, multicomponent structures, and high-throughput materials screening.

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          Most cited references51

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          Generalized Gradient Approximation Made Simple

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            Efficient iterative schemes forab initiototal-energy calculations using a plane-wave basis set

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              Electron-energy-loss spectra and the structural stability of nickel oxide: An LSDA+U study

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                Author and article information

                Journal
                Science
                Science
                American Association for the Advancement of Science (AAAS)
                0036-8075
                1095-9203
                April 30 2020
                May 01 2020
                April 30 2020
                May 01 2020
                : 368
                : 6490
                : 521-526
                Affiliations
                [1 ]Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742, USA.
                [2 ]Department of Mechanical Engineering, Virginia Tech, Blacksburg, VA 24061, USA.
                [3 ]Departments of Civil and Environmental Engineering and Mechanical and Aerospace Engineering, University of California, Los Angeles, CA 90095, USA.
                [4 ]Department of Mechanical Engineering, University of Maryland, College Park, MD 20742, USA.
                [5 ]Department of NanoEngineering, Program of Materials Science and Engineering, University of California San Diego, La Jolla, CA 92093, USA.
                [6 ]Department of Materials Science and Engineering, University of California, Los Angeles, CA 90095, USA.
                [7 ]Center for Materials Innovation, University of Maryland, College Park, MD 20742, USA.
                Article
                10.1126/science.aaz7681
                32355030
                f2964137-7f1b-46cc-86cb-48d805530b0a
                © 2020

                http://www.sciencemag.org/about/science-licenses-journal-article-reuse

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