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      Triboelectric Nanogenerators for Self-Powered Degradation of Chemical Pollutants

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          Abstract

          Environmental and human health is severely threatened by wastewater and air pollution, which contain a broad spectrum of organic and inorganic pollutants. Organic contaminants include dyes, volatile organic compounds (VOCs), medical waste, antibiotics, pesticides, and chemical warfare agents. Inorganic gases such as CO 2, SO 2, and NO x are commonly found in polluted water and air. Traditional methods for pollutant removal, such as oxidation, physicochemical techniques, biotreatment, and enzymatic decomposition, often prove to be inefficient, costly, or energy-intensive. Contemporary solutions like nanofiber-based filters, activated carbon, and plant biomass also face challenges such as generating secondary contaminants and being time-consuming. In this context, triboelectric nanogenerators (TENGs) are emerging as promising alternatives. These devices harvest ambient mechanical energy and convert it to electrical energy, enabling the self-powered degradation of chemical pollutants. This Review summarizes recent progress and challenges in using TENGs as self-powered electrochemical systems (SPECs) for pollutant degradation via photocatalysis or electrocatalysis. The working principles of TENGs are discussed, focusing on their structural flexibility, operational modes, and ability to capture energy from low-frequency mechanical stimuli. The Review concludes with perspectives and suggestions for future research in this field, hoping to inspire further interest and innovation in developing TENG-based SPECs, which represent sustainable and eco-friendly solutions for pollutant treatment.

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          Most cited references200

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          Flexible triboelectric generator

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            Recent developments in photocatalytic water treatment technology: a review.

            In recent years, semiconductor photocatalytic process has shown a great potential as a low-cost, environmental friendly and sustainable treatment technology to align with the "zero" waste scheme in the water/wastewater industry. The ability of this advanced oxidation technology has been widely demonstrated to remove persistent organic compounds and microorganisms in water. At present, the main technical barriers that impede its commercialisation remained on the post-recovery of the catalyst particles after water treatment. This paper reviews the recent R&D progresses of engineered-photocatalysts, photoreactor systems, and the process optimizations and modellings of the photooxidation processes for water treatment. A number of potential and commercial photocatalytic reactor configurations are discussed, in particular the photocatalytic membrane reactors. The effects of key photoreactor operation parameters and water quality on the photo-process performances in terms of the mineralization and disinfection are assessed. For the first time, we describe how to utilize a multi-variables optimization approach to determine the optimum operation parameters so as to enhance process performance and photooxidation efficiency. Both photomineralization and photo-disinfection kinetics and their modellings associated with the photocatalytic water treatment process are detailed. A brief discussion on the life cycle assessment for retrofitting the photocatalytic technology as an alternative waste treatment process is presented. This paper will deliver a scientific and technical overview and useful information to scientists and engineers who work in this field.
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              Advanced Oxidation Processes for Organic Contaminant Destruction Based on the Fenton Reaction and Related Chemistry

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                Author and article information

                Journal
                ACS Omega
                ACS Omega
                ao
                acsodf
                ACS Omega
                American Chemical Society
                2470-1343
                26 December 2024
                14 January 2025
                : 10
                : 1
                : 26-54
                Affiliations
                []Department of Textiles, Merchandising, and Interiors, University of Georgia , Athens, Georgia 30602, United States
                []Department of Materials, University of Manchester , Manchester M13 9PL, United Kingdom
                [§ ]Department of Yarn Engineering, Bangladesh University of Textiles , Dhaka 1208, Bangladesh
                []Department of Design and Merchandising, Oklahoma State University , Stillwater, Oklahoma 74078, United States
                []Department of Textile Engineering, Ahsanullah University of Science and Technology , Dhaka 1208, Bangladesh
                [# ]Department of Apparel Engineering, Bangladesh University of Textiles , Dhaka 1208, Bangladesh
                [g ]Department of Chemistry & Chemical and Biomedical Engineering, University of New Haven , New Haven, Connecticut 30605, United States
                [h ]Department of Fabric Engineering, Bangladesh University of Textiles , Dhaka 1208, Bangladesh
                Author notes
                Author information
                https://orcid.org/0000-0002-3645-9353
                https://orcid.org/0000-0002-0274-1748
                https://orcid.org/0000-0001-8339-0419
                https://orcid.org/0000-0002-1480-1891
                Article
                10.1021/acsomega.4c07889
                11740385
                39829514
                9e4ae0c9-854e-4716-b6df-1974da1978ad
                © 2024 The Authors. Published by American Chemical Society

                Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained ( https://creativecommons.org/licenses/by/4.0/).

                History
                : 27 August 2024
                : 12 December 2024
                : 10 December 2024
                Categories
                Review
                Custom metadata
                ao4c07889
                ao4c07889

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