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      On‐Chip Monolithically Integrated Ultraviolet Low‐Threshold Plasmonic Metal‒Semiconductor Heterojunction Nanolasers

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          Abstract

          The metal‒semiconductor heterojunction is imperative for the realization of electrically driven nanolasers for chip‐level platforms. Progress in developing such nanolasers has hitherto rarely been realized, however, because of their complexity in heterojunction fabrication and the need to use noble metals that are incompatible with microelectronic manufacturing. Most plasmonic nanolasers lase either above a high threshold (10 1‒10 3 MW cm −2) or at a cryogenic temperature, and lasing is possible only after they are removed from the substrate to avoid the large ohmic loss and the low modal reflectivity, making monolithic fabrication impossible. Here, for the first time, record‐low‐threshold, room‐temperature ultraviolet (UV) lasing of plasmon‐coupled core‒shell nanowires that are directly grown on silicon is demonstrated. The naturally formed core‒shell metal‒semiconductor heterostructure of the nanowires leads to a 100‐fold improvement in growth density over previous results. This unprecedentedly high nanowire density creates intense plasmonic resonance, which is outcoupled to the resonant Fabry‒Pérot microcavity. By boosting the emission strength by a factor of 100, the hybrid photonic‒plasmonic system successfully facilitates a record‐low laser threshold of 12 kW cm −2 with a spontaneous emission coupling factor as high as ≈0.32 in the 340‒360 nm range. Such architecture is simple and cost‐competitive for future UV sources in silicon integration.

          Abstract

          By boosting the emission strength by a factor of 100, a new hybrid photonic‒plasmonic architecture is successfully demonstrated to realize low‐threshold room‐temperature UV nanolasers that can be monolithically integrated into silicon. The synergistic engineering of the metal‒semiconductor heterojunction, the modal reflectivity, and the intermodal coupling engender the realization of electrically driven nanolasers.

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          Author and article information

          Contributors
          cclai@gms.ndhu.edu.tw
          Journal
          Adv Sci (Weinh)
          Adv Sci (Weinh)
          10.1002/(ISSN)2198-3844
          ADVS
          Advanced Science
          John Wiley and Sons Inc. (Hoboken )
          2198-3844
          09 August 2023
          October 2023
          : 10
          : 28 ( doiID: 10.1002/advs.v10.28 )
          : 2301493
          Affiliations
          [ 1 ] Department of Physics National Dong Hwa University Hualien 974301 Taiwan
          [ 2 ] Department of Electrical and Computer Engineering University of California Los Angeles CA 90095 USA
          [ 3 ] Institute of Photonics National Yang Ming Chiao Tung University Tainan 711010 Taiwan
          [ 4 ] Institute of Optoelectronics National Chung Hsing University Taichung 402202 Taiwan
          [ 5 ] Department of Optoelectronics and Materials Technology National Taiwan Ocean University Keelung 202301 Taiwan
          [ 6 ] Department of Materials Science and Engineering National Dong Hwa University Hualien 974301 Taiwan
          [ 7 ] Department of Electrical Engineering National Kaohsiung Normal University Kaohsiung 824004 Taiwan
          [ 8 ] Department of Opto‐Electronic Engineering National Dong Hwa University Hualien 974301 Taiwan
          [ 9 ] R&D Center Taiwan Semiconductor Manufacturing Company Hsinchu 300091 Taiwan
          [ 10 ] Department of Dermatology National Taiwan University Hospital and College of Medicine National Taiwan University Taipei 100229 Taiwan
          Author notes
          Author information
          https://orcid.org/0000-0002-8572-116X
          Article
          ADVS6303
          10.1002/advs.202301493
          10558691
          37559172
          886e8a11-2e74-4174-8440-43a72e461b96
          © 2023 The Authors. Advanced Science published by Wiley‐VCH GmbH

          This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.

          History
          : 16 July 2023
          : 07 March 2023
          Page count
          Figures: 6, Tables: 0, Pages: 13, Words: 9836
          Funding
          Funded by: Ministry of Science and Technology, Taiwan , doi 10.13039/501100004663;
          Award ID: MOST 111‐2112‐M‐259‐015
          Award ID: MOST 110‐2112‐M‐259‐008
          Categories
          Research Article
          Research Articles
          Custom metadata
          2.0
          October 6, 2023
          Converter:WILEY_ML3GV2_TO_JATSPMC version:6.3.4 mode:remove_FC converted:06.10.2023

          heterojunction,nanolaser,nanowire,plasmonics,ultraviolet
          heterojunction, nanolaser, nanowire, plasmonics, ultraviolet

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