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      New insights into the electrochemical reduction of carbon dioxide on metallic copper surfaces

      Author(s): , , ,
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      Journal: Energy & Environmental Science
      Publisher: Royal Society of Chemistry (RSC)

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          Ionic liquid-mediated selective conversion of CO₂ to CO at low overpotentials.

          Brian A. Rosen, Amin Salehi-Khojin, Michael R. Thorson … (2011)
          Electroreduction of carbon dioxide (CO(2))--a key component of artificial photosynthesis--has largely been stymied by the impractically high overpotentials necessary to drive the process. We report an electrocatalytic system that reduces CO(2) to carbon monoxide (CO) at overpotentials below 0.2 volt. The system relies on an ionic liquid electrolyte to lower the energy of the (CO(2))(-) intermediate, most likely by complexation, and thereby lower the initial reduction barrier. The silver cathode then catalyzes formation of the final products. Formation of gaseous CO is first observed at an applied voltage of 1.5 volts, just slightly above the minimum (i.e., equilibrium) voltage of 1.33 volts. The system continued producing CO for at least 7 hours at Faradaic efficiencies greater than 96%.
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            Prospects of CO2Utilization via Direct Heterogeneous Electrochemical Reduction

            Devin T. Whipple, Paul Kenis (2010)
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              Electronic structure ofCu2O and CuO

              J Ghijsen, L. H. Tjeng, J. van Elp … (1988)
              Article 0 comments Cited 313 times – based on 0 reviews     Review now
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                Author and article information

                Journal
                Journal ID (publisher-id): EESNBY
                Title: Energy & Environmental Science
                Abbreviated Title: Energy Environ. Sci.
                Publisher: Royal Society of Chemistry (RSC)
                ISSN (Print): 1754-5692
                ISSN (Electronic): 1754-5706
                Publication date Created: 2012
                Publication date (Print): 2012
                Volume: 5
                Issue: 5
                Page: 7050
                Article
                DOI: 10.1039/c2ee21234j
                SO-VID: 7a7afa3d-b498-41eb-899b-2be455edc686
                Copyright © © 2012
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