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      Uncovering Weyl Fermions in the Quantum Limit of NbP

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          Abstract

          The Fermi surface topology of a Weyl semimetal (WSM) depends strongly on the position of the chemical potential. If it resides close to the band touching points (Weyl nodes), as it does in TaAs, separate Fermi surfaces of opposite chirality emerge, leading to novel phenomena such as the chiral magnetic effect. If the chemical potential lies too far from the nodes, however, the chiral Fermi surfaces merge into a single large Fermi surface with no net chirality. This is realized in the WSM NbP, where the Weyl nodes lie far below the Fermi energy and where the transport properties in low magnetic fields show no evidence of chiral Fermi surfaces. Here we show that the behavior of NbP in high magnetic fields is nonetheless dominated by the presence of the Weyl nodes. Torque magnetometry up to 60 tesla reveals a change in the slope of \(\tau/B\) at the quantum limit B\(^\star\) (\(\approx 32\,\rm{T}\)), where the chemical potential enters the \(n=0\) Landau level. Numerical simulations show that this behaviour results from the magnetic field pulling the chemical potential to the chiral \(n=0\) Landau level belonging to the Weyl nodes. These results show that high magnetic fields can uncover topological singularities in the underlying band structure of a potential WSM, and can recover topologically non-trivial experimental properties, even when the position of the chemical potential precludes their observation in zero magnetic field.

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          Topological semimetal and Fermi-arc surface states in the electronic structure of pyrochlore iridates

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            Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal NbP

            , , (2015)
            Recent experiments have revealed spectacular transport properties of conceptually simple semimetals. For example, normal semimetals (e.g. WTe\(_2\)) have started a new trend to realize a large magnetoresistance, which is the change of electrical resistance by an external magnetic field. Weyl semimetal (WSM) is a topological semimetal with massless relativistic electrons as the three-dimensional analogue of graphene and promises exotic transport properties and surface states, which are different from those of the famous topological insulators (TIs). In this letter, we choose to utilize NbP in magneto-transport experiments because its band structure is on assembly of a WSM and a normal semimetal. Such a combination in NbP indeed leads to the observation of remarkable transport properties, an extremely large magnetoresistance of 850,000 % at 1.85 K (250 % at room temperature) in a magnetic field of 9 T without any signs of saturation, and ultrahigh carrier mobility of 5\(\times\)10\(^6\) cm\(^2\) V\(^{-1}\) s\(^{-1}\) accompanied by strong Shubnikov-de Hass (SdH) oscillations. NbP presents a unique example to consequent design the functionality of materials by combining the topological and conventional phases.
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              Negative magnetoresistance without well-defined chirality in the Weyl semimetal TaP

              , , (2016)
              Weyl semimetals (WSMs) are topological quantum states wherein the electronic bands linearly disperse around pairs of nodes, the Weyl points, of fixed (left or right) chirality. The recent discovery of WSM materials triggered an experimental search for the exotic quantum phenomenon known as the chiral anomaly. Via the chiral anomaly nonorthogonal electric and magnetic fields induce a chiral density imbalance that results in an unconventional negative longitudinal magnetoresistance, the chiral magnetic effect. Recent theoretical work suggests that this effect does not require well-defined Weyl nodes. Experimentally however, it remains an open question to what extent it survives when chirality is not well-defined, for example when the Fermi energy is far away from the Weyl points. Here, we establish the detailed Fermi surface topology of the recently identified WSM TaP via a combination of angle-resolved quantum oscillation spectra and band structure calculations. The Fermi surface forms spin-polarized banana-shaped electron and hole pockets attached to pairs of Weyl points. Although the chiral anomaly is therefore ill-defined, we observe a large negative magnetoresistance (NMR) appearing for collinear magnetic and electric fields as observed in other WSMs. In addition, we show experimental signatures indicating that such longitudinal magnetoresistance measurements can be affected by an inhomogeneous current distribution inside the sample in a magnetic field. Our results provide a clear framework how to detect the chiral magnetic effect.
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                Author and article information

                Journal
                22 February 2018
                Article
                1802.08221
                716544f0-8a58-4fd3-94b2-8861772a1318

                http://arxiv.org/licenses/nonexclusive-distrib/1.0/

                History
                Custom metadata
                6 pages including 5 figures
                cond-mat.str-el

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