Sourdough bread (SB) has increased popularity due to health benefits and higher interest in artisan breadmaking due to social isolation during the COVID-19 pandemic. However, quality traits and consumer assessment are still limited to complex laboratory analysis and sensory trials. In this research, new and emerging digital technologies were tested to assess quality traits of SB made from six different flour sources. The results showed that machine learning (ML) models developed to classify the type of wheat used for flours (targets) from near-infrared (NIR) spectroscopy data (Model 1) and a low-cost electronic nose (Model 2) as inputs rendered highly accurate and precise models (96.3% and 99.4%, respectively). Furthermore, ML regression models based on the same inputs for NIR (Model 3) and e-nose (Model 4) were developed to automatically assess 16 volatile aromatic compounds (targets) using GC-MS as ground-truth. To reiterate, models with high accuracy and performance were obtained with correlation (R), determination coefficients (R2), and slope (b) of R = 0.97; R2 = 0.94 and b = 0.99 for Model 3 and R = 0.99; R2 = 0.99 and b = 0.99 for Model 4. The development of low-cost instrumentation and sensors could make possible the accessibility of hardware and software to the industry and artisan breadmakers to assess quality traits and consistency of SB.