Feshbach spectroscopy of an ultracold mixture of $^{85}$Rb and

 $^{133}$Cs

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Abstract

We report the observation of interspecies Feshbach resonances in an optically trapped mixture of $^{85}$Rb and $^{133}$Cs. We measure 14 interspecies features in the lowest spin channels for a magnetic field range from 0 to 700 G and show that they are in good agreement with coupled-channel calculations. The interspecies background scattering length is close to zero over a large range of magnetic fields, permitting the sensitive detection of Feshbach resonances through interspecies thermalisation. Our results confirm the quality of the Rb-Cs potential curves and offer promising starting points for the production of ultracold polar molecules.

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A High Phase-Space-Density Gas of Polar Molecules

P S Julienne, D. S. Jin, J. Ye … (2008)

A quantum gas of ultracold polar molecules, with long-range and anisotropic interactions, would not only enable explorations of a large class of many-body physics phenomena, but could also be used for quantum information processing. We report on the creation of an ultracold dense gas of 40K87Rb polar molecules. Using a single step of STIRAP (STImulated Raman Adiabatic Passage) via two-frequency laser irradiation, we coherently transfer extremely weakly bound KRb molecules to the rovibrational ground state of either the triplet or the singlet electronic ground molecular potential. The polar molecular gas has a peak density of 10^12 cm^-3, and an expansion-determined translational temperature of 350 nK. The polar molecules have a permanent electric dipole moment, which we measure via Stark spectroscopy to be 0.052(2) Debye for the triplet rovibrational ground state and 0.566(17) Debye for the singlet rovibrational ground state. (1 Debye= 3.336*10^-30 C m)

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Quantum-State Controlled Chemical Reactions of Ultracold KRb Molecules

J. Ye, K. -K. Ni, D. Wang … (2009)

How does a chemical reaction proceed at ultralow temperatures? Can simple quantum mechanical rules such as quantum statistics, single scattering partial waves, and quantum threshold laws provide a clear understanding for the molecular reactivity under a vanishing collision energy? Starting with an optically trapped near quantum degenerate gas of polar $^{40}$K$^{87}$Rb molecules prepared in their absolute ground state, we report experimental evidence for exothermic atom-exchange chemical reactions. When these fermionic molecules are prepared in a single quantum state at a temperature of a few hundreds of nanoKelvins, we observe p-wave-dominated quantum threshold collisions arising from tunneling through an angular momentum barrier followed by a near-unity probability short-range chemical reaction. When these molecules are prepared in two different internal states or when molecules and atoms are brought together, the reaction rates are enhanced by a factor of 10 to 100 due to s-wave scattering, which does not have a centrifugal barrier. The measured rates agree with predicted universal loss rates related to the two-body van der Waals length.