The network traffic of data centers (DCs) has increased unprecedentedly with the rapid development of digital economy. However, the data transmission faces security threats in the distributed optical interconnection and intensive interaction of DC networks. In this paper, we propose a chaotic phase noise-like encryption algorithm using geometric shaping (GS) for coherent DC interconnections (DCIs). A GS constellation is used to improve transmission performance, and it is combined with coherent equalization algorithms to improve security performance. Then, a chaotic encryption is designed based on phase noise-like transformation (PNLT). The data are effectively scrambled, and the confusion level of phase can be increased. Finally, 216 Gb/s 8-quadrature amplitude modulation (8-QAM) encrypted data are successfully verified on a 240 km transmission link of DCIs. The results show that this scheme can achieve a bit error rate (BER) performance gain of 1.1 dB and provide a highly compatible solution for realizing security enhanced DCIs.