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      Adaptive on-chip control of nano-optical fields with optoplasmonic vortex nanogates

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          Abstract

          A major challenge for plasmonics as an enabling technology for quantum information processing is the realization of active spatio-temporal control of light on the nanoscale. The use of phase-shaped pulses or beams enforces specific requirements for on-chip integration and imposes strict design limitations. We introduce here an alternative approach, which is based on exploiting the strong sub-wavelength spatial phase modulation in the near-field of resonantly-excited high-Q optical microcavities integrated into plasmonic nanocircuits. Our theoretical analysis reveals the formation of areas of circulating powerflow (optical vortices) in the near-fields of optical microcavities, whose positions and mutual coupling can be controlled by tuning the microcavities parameters and the excitation wavelength. We show that optical powerflow though nanoscale plasmonic structures can be dynamically molded by engineering interactions of microcavity-induced optical vortices with noble-metal nanoparticles. The proposed strategy of re-configuring plasmonic nanocircuits via locally-addressable photonic elements opens the way to develop chip-integrated optoplasmonic switching architectures, which is crucial for implementation of quantum information nanocircuits.

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          Most cited references57

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          Optical Constants of the Noble Metals

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            The Fano resonance in plasmonic nanostructures and metamaterials.

            Since its discovery, the asymmetric Fano resonance has been a characteristic feature of interacting quantum systems. The shape of this resonance is distinctively different from that of conventional symmetric resonance curves. Recently, the Fano resonance has been found in plasmonic nanoparticles, photonic crystals, and electromagnetic metamaterials. The steep dispersion of the Fano resonance profile promises applications in sensors, lasing, switching, and nonlinear and slow-light devices.
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              Demonstration of a spaser-based nanolaser.

              One of the most rapidly growing areas of physics and nanotechnology focuses on plasmonic effects on the nanometre scale, with possible applications ranging from sensing and biomedicine to imaging and information technology. However, the full development of nanoplasmonics is hindered by the lack of devices that can generate coherent plasmonic fields. It has been proposed that in the same way as a laser generates stimulated emission of coherent photons, a 'spaser' could generate stimulated emission of surface plasmons (oscillations of free electrons in metallic nanostructures) in resonating metallic nanostructures adjacent to a gain medium. But attempts to realize a spaser face the challenge of absorption loss in metal, which is particularly strong at optical frequencies. The suggestion to compensate loss by optical gain in localized and propagating surface plasmons has been implemented recently and even allowed the amplification of propagating surface plasmons in open paths. Still, these experiments and the reported enhancement of the stimulated emission of dye molecules in the presence of metallic nanoparticles lack the feedback mechanism present in a spaser. Here we show that 44-nm-diameter nanoparticles with a gold core and dye-doped silica shell allow us to completely overcome the loss of localized surface plasmons by gain and realize a spaser. And in accord with the notion that only surface plasmon resonances are capable of squeezing optical frequency oscillations into a nanoscopic cavity to enable a true nanolaser, we show that outcoupling of surface plasmon oscillations to photonic modes at a wavelength of 531 nm makes our system the smallest nanolaser reported to date-and to our knowledge the first operating at visible wavelengths. We anticipate that now it has been realized experimentally, the spaser will advance our fundamental understanding of nanoplasmonics and the development of practical applications.
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                Author and article information

                Journal
                Opt Express
                Opt Express
                OE
                Optics Express
                Optical Society of America
                1094-4087
                24 October 2011
                24 October 2011
                24 October 2012
                : 19
                : 22
                : 22305-22315
                Affiliations
                [1 ]Department of Chemistry & The Photonics Center, Boston University, Boston, MA 02215, USA
                [2 ] sboriskina@ 123456gmail.com
                [3 ] bmr@ 123456bu.edu
                Article
                152825
                10.1364/OE.19.022305
                3298770
                22109072
                24b9a4c7-1b9e-4280-9ba1-fcde1dbd5e99
                ©2011 Optical Society of America

                This is an open-access article distributed under the terms of the Creative Commons Attribution-Noncommercial-No Derivative Works 3.0 Unported License, which permits download and redistribution, provided that the original work is properly cited. This license restricts the article from being modified or used commercially.

                History
                : 15 August 2011
                : 15 September 2011
                : 15 September 2011
                Funding
                Funded by: National Institutes of Health
                Award ID: 5R01CA138509-03
                Funded by: National Science Foundation
                Award ID: CBET-0853798
                Award ID: CBET-0953121
                Funded by: EU COST Action
                Award ID: MP0702
                Categories
                Research-Article
                Custom metadata
                True
                12

                Ophthalmology & Optometry
                (250.6715) switching,(140.3945) microcavities,(230.4555) coupled resonators,(250.5403) plasmonics,(240.6680) surface plasmons

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