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      Lanthanide organic–inorganic hybrids based on functionalized metal–organic frameworks (MOFs) for a near-UV white LED

      Author(s): ,
      Publication date (Print):
      Journal: Chem. Commun.
      Publisher: Royal Society of Chemistry (RSC)

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          Abstract

          A novel near-UV white LED based on lanthanide organic–inorganic hybrid material is realized through postsynthetically modified MOFs and MOF-based polymers. The hybrids materials have high quantum yield and satisfactory luminescence stability; the assembled white LED has tuneable correlated color temperature and high color rendering index.

          Abstract

          A novel near-UV white LED based on lanthanide organic–inorganic hybrid material is realized through postsynthetically modified MOFs and MOF-based polymers. The hybrids materials have high quantum yield and satisfactory luminescence stability; the assembled white LED has tuneable correlated color temperature and high color rendering index.

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          Most cited references34

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          Lanthanide-based luminescent hybrid materials.

          Koen Binnemans (2009)
          Article 0 comments Cited 473 times – based on 0 reviews     Review now
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            Luminescent multifunctional lanthanides-based metal-organic frameworks.

            Maria João Rocha, Luís Carlos, Filipe Paz … (2011)
            Metal-organic frameworks based on trivalent lanthanides (LnMOFs) are a very promising class of materials for addressing the challenges in engineering of luminescent centres. Lanthanide-bearing phosphors find numerous applications in lighting, optical communications, photonics and biomedical devices. In this critical review we discuss the potential of LnMOFs as multifunctional systems, which combine light emission with properties such as microporosity, magnetism, chirality, molecule and ion sensing, catalysis and activity as multimodal imaging contrast agents. We argue that these materials present a unique chance of observing synergy between several of these properties, such as the coupling between photoluminescence and magnetism. Moreover, an integrated approach towards the design of efficient, stable, cheap, environmentally-friendly and multifunctional luminescent LnMOFs is still missing. Although research into LnMOFs is at its early stage and much basic knowledge is still needed, the field is ripe for new ideas, which will enable sensor devices and photonic prototypes to become a commercial reality (81 references).
            Article 0 comments Cited 338 times – based on 0 reviews     Review now
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              Lanthanide-containing light-emitting organic-inorganic hybrids: a bet on the future.

              Luís Carlos, Luisa Ferreira, Verónica de Zea Bermudez … (2009)
              Interest in lanthanide-containing organic-inorganic hybrids has grown considerably during the last decade, with the concomitant fabrication of materials with tunable attributes offering modulated properties. The potential of these materials relies on exploiting the synergy between the intrinsic characteristics of sol-gel derived hosts (highly controlled purity, versatile shaping and patterning, excellent optical quality, easy control of the refractive index, photosensitivity, encapsulation of large amounts of isolated emitting centers protected by the host) and the luminescence features of trivalent lanthanide ions (high luminescence quantum yield, narrow bandwidth, long-lived emission, large Stokes shifts, ligand-dependent luminescence sensitization). Promising applications may be envisaged, such as light-emitting devices, active waveguides in the visible and near-IR spectral regions, active coatings, and bio-medical actuators and sensors, opening up exciting directions in materials science and related technologies with significant implications in the integration, miniaturization, and multifunctionalization of devices. This review provides an overview of the latest advances in Ln(3+)-containing siloxane-based hybrids, with emphasis on the different possible synthetic strategies, photoluminescence features, empirical determination.
              Article 0 comments Cited 155 times – based on 0 reviews     Review now
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                Author and article information

                Journal
                Journal ID (publisher-id): CHCOFS
                Title: Chem. Commun.
                Abbreviated Title: Chem. Commun.
                Publisher: Royal Society of Chemistry (RSC)
                ISSN (Print): 1359-7345
                ISSN (Electronic): 1364-548X
                Publication date Created: 2014
                Publication date (Print): 2014
                Volume: 50
                Issue: 97
                Pages: 15443-15446
                Article
                DOI: 10.1039/C4CC07852G
                SO-VID: 5f63103a-7b0a-42cb-83d0-528cf068bc9a
                Copyright © © 2014
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