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      Long-range interactions between polar bialkali ground-state molecules in arbitrary vibrational levels

      1 , 1 , 1 , 1 , 1
      The Journal of Chemical Physics
      AIP Publishing

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          Coherent population transfer among quantum states of atoms and molecules

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            Is Open Access

            A High Phase-Space-Density Gas of Polar Molecules

            A quantum gas of ultracold polar molecules, with long-range and anisotropic interactions, would not only enable explorations of a large class of many-body physics phenomena, but could also be used for quantum information processing. We report on the creation of an ultracold dense gas of 40K87Rb polar molecules. Using a single step of STIRAP (STImulated Raman Adiabatic Passage) via two-frequency laser irradiation, we coherently transfer extremely weakly bound KRb molecules to the rovibrational ground state of either the triplet or the singlet electronic ground molecular potential. The polar molecular gas has a peak density of 10^12 cm^-3, and an expansion-determined translational temperature of 350 nK. The polar molecules have a permanent electric dipole moment, which we measure via Stark spectroscopy to be 0.052(2) Debye for the triplet rovibrational ground state and 0.566(17) Debye for the singlet rovibrational ground state. (1 Debye= 3.336*10^-30 C m)
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              Theoretical progress in many-body physics with ultracold dipolar gases

              M. Baranov (2008)
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                Author and article information

                Journal
                The Journal of Chemical Physics
                The Journal of Chemical Physics
                AIP Publishing
                0021-9606
                1089-7690
                June 07 2015
                June 07 2015
                : 142
                : 21
                : 214303
                Affiliations
                [1 ]Laboratoire Aimé Cotton, CNRS/Université Paris-Sud/ENS-Cachan, Bât. 505, Campus d’Orsay, 91405 Orsay, France
                Article
                10.1063/1.4921622
                7dc9ab0a-8808-4350-80a3-75eb85fa8f80
                © 2015
                History

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