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Recent advances in process engineering and upcoming applications of metal–organic frameworks
review-article
UnJin Ryu
a
,
1 ,
Seohyeon Jee
a
,
1 ,
Purna Chandra Rao
b
,
1 ,
Jeeyoung Shin
c
,
d ,
Changhyun Ko
d
,
e ,
Minyoung Yoon
b
,
* ,
Kyo Sung Park
f
,
* ,
Kyung Min Choi
a
,
d
,
*
18 September 2020
Metal–organic framework,
Commercialization,
Mass production,
Future applications,
Shaping,
Dispersion,
MOF, metal–organic framework,
ZIF, zeolitic imidazolate framework,
DMF, N,N-Dimethyl formamide,
DEF, N,N-Diethyl formamide,
DMA, Dimethylacetamide,
TEA, Triethylamine,
STY, space–time yield, grams of MOF per cubic meter of reaction mixture per day of synthesis ,
NMP, N-methyl-2-pyrrolidone,
CNG, compressed natural gas,
PEI, Polyetherimide,
PS, Polystyrene,
PVA, Polyvinyl alcohol,
MRA, mesoporous ρ-alumina,
ABS, acrylonitril-butadiene-styrene,
CA, Cellulose-acetate,
PXRD, Powder x-ray diffraction,
PVC, Polyvinylchloride,
PVF, Polyvinylformal,
PVB, Polyvinyl Butyral,
DLS, Dynamic light scattering,
BET, Brunauer–Emmett–Teller,
PEG-CCM, polyethylene-glycol-modified mono-functional curcumin,
MB, methylene blue,
DDM, n-dodecyl β-D-maltoside,
ECS, Extrusion-crushing-sieving,
TIPS-HoP, Thermally induced phase separation-hot pressing,
PM, Particulate matter,
VOC, Volatile organic compound,
CWA, Chemical warfare agent,
PPC, Polypropylene/polycarbonate,
PAN, Polyacrylonitrile,
SEM, Scanning electron microscope,
SBU, Secondary building unit,
DFT, Density functional theory,
SALI, Solvent assisted ligand incorporation,
FT-IR, Fourier-transform infrared spectroscopy,
NMR, Nuclear magnetic resonance,
DRIFTS, Diffuse reflectance infrared fourier transform spectroscopy,
XPS, X-ray photoelectron spectroscopy,
SCXRD, Single-crystal X-ray diffraction,
CWC, Chemical weapons convention,
POM, Polyoxometalate,
DMMP, Dimethyl methylphosphonate,
GC–MS, Gas chromatography–mass spectrometry,
EXAFS, Extended X-ray absorption fine structure,
MMP, Methyl methylphosphonate,
DIFP, Diisopropylfluorophosphate,
MVTR, Moisture vapor transport rate,
CEES, 2-Chloroethyl ethyl sulfide,
DCP, Diethylchlorophosphonate,
DFP, Diisopropyl fluorophosphate,
ROS, Reactive oxygen species,
E. Coli, Escherichia coli,
MRSA, Methicillin-resistant staphylococcus aureus,
MIC, Minimum inhibitory concentration,
MBC, Minimum bactericidal concentration,
PSM, Post-synthetic modification,
CNF, Cellulose nanofiber,
GRGDS, Gly-Arg-Gly-Asp-Ser,
Fn, Fusobacterium nucleatum,
Pg, Porphyromonas gingivalis,
PEMFCs, Proton-exchange membrane fuel cells,
SSEs, Solid-state electrolytes,
MOGs, Metal-organic gels,
LIBs, Lithium-ion batteries,
SIBs, Sodium-ion batteries,
hXAS, Hard X-ray absorption spectroscopy,
sXAS, Soft X-ray absorption spectroscopy,
EDLCs, Electrochemical double-layer capacitors,
PANI, Polyaniline,
ILDs, Interlayer dielectrics,
ITRS, International technology roadmap for semiconductors,
CVD, Chemical vapor deposition,
MIM, Metal-insulator–metal,
LMOF, Luminescent metal–organic framework,
UPS, Ultraviolet photoelectron spectroscopy,
EPA, Environmental protection agency,
WHO, World health organization,
LOD, Limit of detection,
TNT, 2,4,6-trinitrotoluene,
TNP, 2,4,6-trinitrophenol,
2,4-DNT, 2,4-dinitrotoluene,
4-NP, 4-nitrophenol,
RDX, 1,3,5-trinitro-1,3,5-triazinane,
LED, Light-emitting diode,
WLED, White light emitting diode,
CIE, Commission international ed’Eclairage
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Graphical abstract
Highlights
Abstract
Progress in metal–organic frameworks (MOFs) has advanced from fundamental chemistry to engineering processes and applications, resulting in new industrial opportunities. The unique features of MOFs, such as their permanent porosity, high surface area, and structural flexibility, continue to draw industrial interest outside the traditional MOF field, both to solve existing challenges and to create new businesses. In this context, diverse research has been directed toward commercializing MOFs, but such studies have been performed according to a variety of individual goals. Therefore, there have been limited opportunities to share the challenges, goals, and findings with most of the MOF field. In this review, we examine the issues and demands for MOF commercialization and investigate recent advances in MOF process engineering and applications. Specifically, we discuss the criteria for MOF commercialization from the views of stability, producibility, regulations, and production cost. This review covers progress in the mass production and formation of MOFs along with future applications that are not currently well known but have high potential for new areas of MOF commercialization.
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Author and article information
metal–organic framework,commercialization,mass production,future applications,shaping,dispersion,mof, metal–organic framework,zif, zeolitic imidazolate framework,dmf, n,n-dimethyl formamide,def, n,n-diethyl formamide,dma, dimethylacetamide,tea, triethylamine,sty, space–time yield, grams of mof per cubic meter of reaction mixture per day of synthesis,nmp, n-methyl-2-pyrrolidone,cng, compressed natural gas,pei, polyetherimide,ps, polystyrene,pva, polyvinyl alcohol,mra, mesoporous ρ-alumina,abs, acrylonitril-butadiene-styrene,ca, cellulose-acetate,pxrd, powder x-ray diffraction,pvc, polyvinylchloride,pvf, polyvinylformal,pvb, polyvinyl butyral,dls, dynamic light scattering,bet, brunauer–emmett–teller,peg-ccm, polyethylene-glycol-modified mono-functional curcumin,mb, methylene blue,ddm, n-dodecyl β-d-maltoside,ecs, extrusion-crushing-sieving,tips-hop, thermally induced phase separation-hot pressing,pm, particulate matter,voc, volatile organic compound,cwa, chemical warfare agent,ppc, polypropylene/polycarbonate,pan, polyacrylonitrile,sem, scanning electron microscope,sbu, secondary building unit,dft, density functional theory,sali, solvent assisted ligand incorporation,ft-ir, fourier-transform infrared spectroscopy,nmr, nuclear magnetic resonance,drifts, diffuse reflectance infrared fourier transform spectroscopy,xps, x-ray photoelectron spectroscopy,scxrd, single-crystal x-ray diffraction,cwc, chemical weapons convention,pom, polyoxometalate,dmmp, dimethyl methylphosphonate,gc–ms, gas chromatography–mass spectrometry,exafs, extended x-ray absorption fine structure,mmp, methyl methylphosphonate,difp, diisopropylfluorophosphate,mvtr, moisture vapor transport rate,cees, 2-chloroethyl ethyl sulfide,dcp, diethylchlorophosphonate,dfp, diisopropyl fluorophosphate,ros, reactive oxygen species,e. coli, escherichia coli,mrsa, methicillin-resistant staphylococcus aureus,mic, minimum inhibitory concentration,mbc, minimum bactericidal concentration,psm, post-synthetic modification,cnf, cellulose nanofiber,grgds, gly-arg-gly-asp-ser,fn, fusobacterium nucleatum,pg, porphyromonas gingivalis,pemfcs, proton-exchange membrane fuel cells,sses, solid-state electrolytes,mogs, metal-organic gels,libs, lithium-ion batteries,sibs, sodium-ion batteries,hxas, hard x-ray absorption spectroscopy,sxas, soft x-ray absorption spectroscopy,edlcs, electrochemical double-layer capacitors,pani, polyaniline,ilds, interlayer dielectrics,itrs, international technology roadmap for semiconductors,cvd, chemical vapor deposition,mim, metal-insulator–metal,lmof, luminescent metal–organic framework,ups, ultraviolet photoelectron spectroscopy,epa, environmental protection agency,who, world health organization,lod, limit of detection,tnt, 2,4,6-trinitrotoluene,tnp, 2,4,6-trinitrophenol,2,4-dnt, 2,4-dinitrotoluene,4-np, 4-nitrophenol,rdx, 1,3,5-trinitro-1,3,5-triazinane,led, light-emitting diode,wled, white light emitting diode,cie, commission international ed’eclairage
metal–organic framework, commercialization, mass production, future applications, shaping, dispersion, mof, metal–organic framework, zif, zeolitic imidazolate framework, dmf, n,n-dimethyl formamide, def, n,n-diethyl formamide, dma, dimethylacetamide, tea, triethylamine, sty, space–time yield, grams of mof per cubic meter of reaction mixture per day of synthesis, nmp, n-methyl-2-pyrrolidone, cng, compressed natural gas, pei, polyetherimide, ps, polystyrene, pva, polyvinyl alcohol, mra, mesoporous ρ-alumina, abs, acrylonitril-butadiene-styrene, ca, cellulose-acetate, pxrd, powder x-ray diffraction, pvc, polyvinylchloride, pvf, polyvinylformal, pvb, polyvinyl butyral, dls, dynamic light scattering, bet, brunauer–emmett–teller, peg-ccm, polyethylene-glycol-modified mono-functional curcumin, mb, methylene blue, ddm, n-dodecyl β-d-maltoside, ecs, extrusion-crushing-sieving, tips-hop, thermally induced phase separation-hot pressing, pm, particulate matter, voc, volatile organic compound, cwa, chemical warfare agent, ppc, polypropylene/polycarbonate, pan, polyacrylonitrile, sem, scanning electron microscope, sbu, secondary building unit, dft, density functional theory, sali, solvent assisted ligand incorporation, ft-ir, fourier-transform infrared spectroscopy, nmr, nuclear magnetic resonance, drifts, diffuse reflectance infrared fourier transform spectroscopy, xps, x-ray photoelectron spectroscopy, scxrd, single-crystal x-ray diffraction, cwc, chemical weapons convention, pom, polyoxometalate, dmmp, dimethyl methylphosphonate, gc–ms, gas chromatography–mass spectrometry, exafs, extended x-ray absorption fine structure, mmp, methyl methylphosphonate, difp, diisopropylfluorophosphate, mvtr, moisture vapor transport rate, cees, 2-chloroethyl ethyl sulfide, dcp, diethylchlorophosphonate, dfp, diisopropyl fluorophosphate, ros, reactive oxygen species, e. coli, escherichia coli, mrsa, methicillin-resistant staphylococcus aureus, mic, minimum inhibitory concentration, mbc, minimum bactericidal concentration, psm, post-synthetic modification, cnf, cellulose nanofiber, grgds, gly-arg-gly-asp-ser, fn, fusobacterium nucleatum, pg, porphyromonas gingivalis, pemfcs, proton-exchange membrane fuel cells, sses, solid-state electrolytes, mogs, metal-organic gels, libs, lithium-ion batteries, sibs, sodium-ion batteries, hxas, hard x-ray absorption spectroscopy, sxas, soft x-ray absorption spectroscopy, edlcs, electrochemical double-layer capacitors, pani, polyaniline, ilds, interlayer dielectrics, itrs, international technology roadmap for semiconductors, cvd, chemical vapor deposition, mim, metal-insulator–metal, lmof, luminescent metal–organic framework, ups, ultraviolet photoelectron spectroscopy, epa, environmental protection agency, who, world health organization, lod, limit of detection, tnt, 2,4,6-trinitrotoluene, tnp, 2,4,6-trinitrophenol, 2,4-dnt, 2,4-dinitrotoluene, 4-np, 4-nitrophenol, rdx, 1,3,5-trinitro-1,3,5-triazinane, led, light-emitting diode, wled, white light emitting diode, cie, commission international ed’eclairage