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      Aluminum Plasmonics Enriched Ultraviolet GaN Photodetector with Ultrahigh Responsivity, Detectivity, and Broad Bandwidth

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          Abstract

          Plasmonics have been well investigated on photodetectors, particularly in IR and visible regimes. However, for a wide range of ultraviolet (UV) applications, plasmonics remain unavailable mainly because of the constrained optical properties of applicable plasmonic materials in the UV regime. Therefore, an epitaxial single‐crystalline aluminum (Al) film, an abundant metal with high plasma frequency and low intrinsic loss is fabricated, on a wide bandgap semiconductive gallium nitride (GaN) to form a UV photodetector. By deliberately designing a periodic nanohole array in this Al film, localized surface plasmon resonance and extraordinary transmission are enabled; hence, the maximum responsivity (670 A W −1) and highest detectivity (1.48 × 10 15 cm Hz 1/2 W −1) is obtained at the resonance wavelength of 355 nm. In addition, owing to coupling among nanoholes, the bandwidth expands substantially, encompassing the entire UV range. Finally, a Schottky contact is formed between the single‐crystalline Al nanohole array and the GaN substrate, resulting in a fast temporal response with a rise time of 51 ms and a fall time of 197 ms. To the best knowledge, the presented detectivity is the highest compared with those of other reported GaN photodetectors.

          Abstract

          Aluminum plasmonics is merged as an advancement tool to boost GaN a superior complementary metal oxide semiconductor (CMOS) compatible UV photodetector. By introducing a single‐crystalline Al nanohole array on a GaN substrate, it enables ultraviolet plasmons and Schottky barrier, and thus demonstrates excellent performance in entire UV regime: maximum responsivity (670 A W −1), highest detectivity (1.48 × 10 15 cm Hz 1/2 W −1), and fast temporal response.

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          Author and article information

          Contributors
          gwo@phys.nthu.edu.tw
          tjyen@mx.nthu.edu.tw
          Journal
          Adv Sci (Weinh)
          Adv Sci (Weinh)
          10.1002/(ISSN)2198-3844
          ADVS
          Advanced Science
          John Wiley and Sons Inc. (Hoboken )
          2198-3844
          17 November 2020
          December 2020
          : 7
          : 24 ( doiID: 10.1002/advs.v7.24 )
          : 2002274
          Affiliations
          [ 1 ] Department of Materials Science and Engineering National Tsing Hua University Hsinchu 300 Taiwan
          [ 2 ] Institute of NanoEngineering and MicroSystems National Tsing Hua University Hsinchu 300 Taiwan
          [ 3 ] Research Centre for Applied Science Academia Sinica Taipei 115‐29 Taiwan
          [ 4 ] Department of Physics National Tsing Hua University Hsinchu 300 Taiwan
          Author notes
          Author information
          https://orcid.org/0000-0002-0826-8680
          https://orcid.org/0000-0002-3013-0477
          https://orcid.org/0000-0003-3613-699X
          Article
          ADVS2053
          10.1002/advs.202002274
          7740085
          29f9379c-fb67-4950-a857-f8ea5547e597
          © 2020 The Authors. Published by Wiley‐VCH GmbH

          This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.

          History
          : 16 June 2020
          : 17 August 2020
          Page count
          Figures: 6, Tables: 1, Pages: 7, Words: 4620
          Funding
          Funded by: High Entropy Materials Center
          Funded by: Featured Areas Research Center Program
          Funded by: Higher Education Sprout Project
          Funded by: Ministry of Education , open-funder-registry 10.13039/100009950;
          Funded by: MOST , open-funder-registry 10.13039/100007225;
          Award ID: 109‐2634‐F‐007‐024
          Award ID: 107‐2923‐M‐007‐004‐MY3
          Award ID: 108‐2119‐M‐007‐008‐ 108‐3116‐F‐002‐ 107‐2221‐E‐007‐016‐MY3
          Categories
          Communication
          Communications
          Custom metadata
          2.0
          December 16, 2020
          Converter:WILEY_ML3GV2_TO_JATSPMC version:5.9.5 mode:remove_FC converted:16.12.2020

          epitaxial aluminum film,gan,uv photodetection,uv plasmonics

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